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dc.contributor.CRUESPUniversidade Estadual de Campinaspt_BR
dc.typeArtigo de periódicopt_BR
dc.titleCharge-Tagged Acetate Ligands As Mass Spectrometry Probes for Metal Complexes Investigations: Applications in Suzuki and Heck Phosphine-Free Reactionspt_BR
dc.contributor.authorOliveira, FFDpt_BR
dc.contributor.authordos Santos, MRpt_BR
dc.contributor.authorLalli, PMpt_BR
dc.contributor.authorSchmidt, EMpt_BR
dc.contributor.authorBakuzis, Ppt_BR
dc.contributor.authorLapis, AAMpt_BR
dc.contributor.authorMonteiro, ALpt_BR
dc.contributor.authorEberlin, MNpt_BR
dc.contributor.authorNeto, BADpt_BR
unicamp.author.emaileberlin@iqm.unicamp.brpt_BR
unicamp.author.emailbrenno.ipi@gmail.compt_BR
unicamp.authorLalli, Priscila M. Schmidt, Eduardo M. Eberlin, Marcos N. Univ Estadual Campinas, ThoMSon Mass Spectrometry Lab, Campinas, SP, Brazilpt_BR
unicamp.authorOliveira, Felipe F. D. dos Santos, Marcelo R. Bakuzis, Peter Neto, Brenno A. D. Univ Brasilia, Lab Med & Technol Chem, Inst Chem, BR-70904970 Brasilia, DF, Brazilpt_BR
unicamp.authorLapis, Alexandre A. M. Univ Fed Fronteira Sul, Chapeco, SC, Brazilpt_BR
unicamp.authorMonteiro, Adriano L. Univ Fed Rio Grande do Sul, Lab Mol Catalysis, Inst Chem, BR-91501970 Porto Alegre, RS, Brazilpt_BR
dc.subject.wosCross-coupling Reactionspt_BR
dc.subject.wosImidazolium Ionic Liquidspt_BR
dc.subject.wosElectrospray-ionizationpt_BR
dc.subject.wosPalladium(0) Complexespt_BR
dc.subject.wosOxidative Additionpt_BR
dc.subject.wosCarbene Complexespt_BR
dc.subject.wosGas-phasept_BR
dc.subject.wosMechanismpt_BR
dc.subject.wosCatalysispt_BR
dc.subject.wosMediapt_BR
dc.description.abstractAn acetate anion bearing an imidazolium cation as its charge tag was reacted with M(OAc)(2) complexes (where M = Ni, Cu, and Pd; in situ reaction) to form members of a new class of charge-tagged metal complexes. The formation of these unprecedented precatalysts with potential for cross-coupling reactions was confirmed by electrospray ionization (and tandem) mass spectrometry. The catalytic performance of the palladium complex was tested in Heck and Suzuki cross-coupling reactions, often with superior activity and yields as compared with Pd(OAc)(2).pt
dc.relation.ispartofJournal Of Organic Chemistrypt_BR
dc.relation.ispartofabbreviationJ. Org. Chem.pt_BR
dc.publisher.cityWashingtonpt_BR
dc.publisher.countryEUApt_BR
dc.publisherAmer Chemical Socpt_BR
dc.date.issued2011pt_BR
dc.date.monthofcirculationDEC 16pt_BR
dc.identifier.citationJournal Of Organic Chemistry. Amer Chemical Soc, v. 76, n. 24, n. 10140, n. 10147, 2011.pt_BR
dc.language.isoenpt_BR
dc.description.volume76pt_BR
dc.description.issuenumber24pt_BR
dc.description.firstpage10140pt_BR
dc.description.lastpage10147pt_BR
dc.rightsfechadopt_BR
dc.sourceWeb of Sciencept_BR
dc.identifier.issn0022-3263pt_BR
dc.identifier.wosidWOS:000297715900026pt_BR
dc.identifier.doi10.1021/jo201990npt_BR
dc.description.sponsorshipCoordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES)pt_BR
dc.description.sponsorshipConselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)pt_BR
dc.description.sponsorshipFINEP-MCTpt_BR
dc.description.sponsorshipFINATECpt_BR
dc.description.sponsorshipFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)pt_BR
dc.description.sponsorshipFAPDFpt_BR
dc.description.sponsorshipDPP-UnBpt_BR
dc.description.sponsorshipANP-PETROBRASpt_BR
dc.description.sponsorship1Coordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES)pt_BR
dc.description.sponsorship1Conselho Nacional de Desenvolvimento Científico e Tecnológico (CNPq)pt_BR
dc.description.sponsorship1Fundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)pt_BR
dc.date.available2014-07-30T16:52:11Z
dc.date.available2015-11-26T16:40:06Z-
dc.date.accessioned2014-07-30T16:52:11Z
dc.date.accessioned2015-11-26T16:40:06Z-
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dc.identifier.urihttp://www.repositorio.unicamp.br/jspui/handle/REPOSIP/62945
dc.identifier.urihttp://repositorio.unicamp.br/jspui/handle/REPOSIP/62945-
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