Please use this identifier to cite or link to this item:
Type: Artigo de periódico
Title: Search For Spin-lattice Coupling Mediated By Itinerant Electrons: Synchrotron X-ray Diffraction And Raman Scattering From Gd Al3
Author: Garcia-Flores A.F.
Malachias A.
Granado E.
Fisk Z.
Abstract: The coupling among the spin degree of freedom and the atomic displacements in intermetallic Gd Al3 was investigated by means of synchrotron x-ray diffraction and polarized Raman scattering. In this compound, the Gd 4 f7 shell is spherical and the spin-lattice coupling provides a fingerprint of the exchange mechanism and degree of magnetic correlations. X-ray diffraction shows nonresonant symmetry-forbidden charge Bragg peaks below the long-range magnetic ordering temperature TN =18 K, revealing a symmetry-lowering crystal lattice transition associated with Gd displacements, consistent with a Ruderman-Kittel-Kasuya-Yosida mechanism for the magnetic coupling. Raman scattering in fresh broken surfaces shows phonons with conventional frequency behavior, while naturally grown and polished surfaces present frequency anomalies below T* ∼50 K. Such anomalies are possibly due to a modulation of the magnetic energy by the lattice vibrations in a strongly spin-correlated paramagnetic phase. Such interpretation implies that the spin-phonon coupling in metals may depend on the surface conditions. A fully spin-correlated state immediately above TN is inferred from our results in this frustrated system. © 2008 The American Physical Society.
Rights: aberto
Identifier DOI: 10.1103/PhysRevB.77.024414
Date Issue: 2008
Appears in Collections:Unicamp - Artigos e Outros Documentos

Files in This Item:
File SizeFormat 
2-s2.0-38349112924.pdf1.34 MBAdobe PDFView/Open

Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.